TY - JOUR
T1 - Tannin-furanic foams used as biomaterial substrates for SERS sensing in possible wastewater filter applications
AU - Sabathi, G.
AU - Reyer, A.
AU - Cefarin, N.
AU - Sepperer, T.
AU - Eckardt, J.
AU - Neubauer, J.
AU - Jan Wendisch, F.
AU - D'Amico, F.
AU - Vaccari, L.
AU - Tondi, G.
AU - Musso, M.
N1 - Cited By :4
Export Date: 14 December 2023
Correspondence Address: Sabathi, G.; Department Chemistry and Physics of Materials, Jakob-Haringerstraße 2A, Austria; email: [email protected]
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PY - 2021/11/23
Y1 - 2021/11/23
N2 - Simple substrates for surface enhanced Raman spectroscopy (SERS), producible in a cost-efficient way, are of growing interest both for scientific and for environmental applications. In this study, we demonstrate the use of three types of bio-based tannin-furanic rigid foams as precursor materials for SERS substrates. Coated with a silver layer, these substrates allowed the detection of several well-known analytes in the mM regime by Raman spectroscopy. Specific optimization of the standard tannin-furanic foam morphology by tuning the chemical synthesis led to a smaller and more homogeneously distributed pore structure, supplying more active hot spot areas. Thus, we obtained a significant increase and a lower relative standard deviation (RSD) of the SERS signal recorded over the mapped SERS substrate area, for several analytes, in particular for Malachite Green dye. This work represents a feasibility study opening several potential applications of this biopolymers in fields such as the detection of water pollutants, virtually combining filtration and SERS capabilities driven by a controlled porosity.
AB - Simple substrates for surface enhanced Raman spectroscopy (SERS), producible in a cost-efficient way, are of growing interest both for scientific and for environmental applications. In this study, we demonstrate the use of three types of bio-based tannin-furanic rigid foams as precursor materials for SERS substrates. Coated with a silver layer, these substrates allowed the detection of several well-known analytes in the mM regime by Raman spectroscopy. Specific optimization of the standard tannin-furanic foam morphology by tuning the chemical synthesis led to a smaller and more homogeneously distributed pore structure, supplying more active hot spot areas. Thus, we obtained a significant increase and a lower relative standard deviation (RSD) of the SERS signal recorded over the mapped SERS substrate area, for several analytes, in particular for Malachite Green dye. This work represents a feasibility study opening several potential applications of this biopolymers in fields such as the detection of water pollutants, virtually combining filtration and SERS capabilities driven by a controlled porosity.
KW - Biopolymers
KW - Flavonoids
KW - Morphology
KW - Raman spectroscopy
KW - Substrates
KW - Tannins
KW - Water filtration
KW - Water pollution
KW - Analytes
KW - Bio-based
KW - Cost-efficient
KW - Environmental applications
KW - Filter applications
KW - Precursor materials
KW - Rigid foams
KW - Silver layer
KW - Simple++
KW - Surface enhanced Raman spectroscopy
KW - Pore structure
UR - https://www.mendeley.com/catalogue/297501c7-a334-3599-8de4-42984ff38e15/
U2 - 10.1088/2053-1591/ac3586
DO - 10.1088/2053-1591/ac3586
M3 - Article
SN - 2053-1591
VL - 8
JO - Mater. Res. Express
JF - Mater. Res. Express
IS - 11
ER -